dc.contributor.author | Harde, H. | |
dc.contributor.author | Katzenellenbogen, N. | |
dc.contributor.author | Grischkowsky, D. | |
dc.date.accessioned | 2015-10-16T20:48:23Z | |
dc.date.available | 2015-10-16T20:48:23Z | |
dc.date.issued | 1995-02-20 | |
dc.identifier | okds_Grischkowsky_PRL_1995-02-20 | |
dc.identifier.citation | Harde, H., Katzenellenbogen, N., & Grischkowsky, D. (1995). Line-shape transition of collision broadened lines. Physical Review Letters, 74(8), 1307-1310. https://doi.org/10.1103/PhysRevLett.74.1307 | |
dc.identifier.uri | https://hdl.handle.net/11244/19912 | |
dc.description.abstract | Using the newly developed technique of THz time-domain spectroscopy, we have measured the far-wing absorption line profile of the ensemble of collision broadened ground state rotational lines of methylchloride vapor out to more than 200 linewidths from resonance, corresponding to frequency offsets as much as 5X the resonant frequency. On these far wings the measured absorption is approximately an order of magnitude less than that predicted by the van Vleck-Weisskopf theory. Our observations show that at higher frequencies a transition occurs from the regime of the van Vleck- Weisskopf theory to the regime of the Lorentz theory. | |
dc.format | application/pdf | |
dc.language | en_US | |
dc.publisher | American Physical Society | |
dc.rights | This material has been previously published. In the Oklahoma State University Library's institutional repository this version is made available through the open access principles and the terms of agreement/consent between the author(s) and the publisher. The permission policy on the use, reproduction or distribution of the material falls under fair use for educational, scholarship, and research purposes. Contact Digital Resources and Discovery Services at lib-dls@okstate.edu or 405-744-9161 for further information. | |
dc.title | Line-shape transition of collision broadened lines | |
osu.filename | okds_Grischkowsky_PRL_1995-02-20.pdf | |
dc.description.peerreview | Peer reviewed | |
dc.identifier.doi | 10.1103/PhysRevLett.74.1307 | |
dc.description.department | Electrical and Computer Engineering | |
dc.type.genre | Article | |
dc.type.material | Text | |
dc.subject.keywords | collision broadened lines | |
dc.subject.keywords | time-domain spectroscopy | |
dc.subject.keywords | far-wing absorption line profile | |
dc.subject.keywords | ground state rotational lines | |
dc.subject.keywords | line-shape transition | |
dc.subject.keywords | methylchloride vapor | |
dc.subject.keywords | frequency offsets | |
dc.subject.keywords | resonant frequency | |
dc.subject.keywords | van vleck-weisskopf theory | |
dc.subject.keywords | lorentz theory | |